Description
Title: Programmable Thermoresponsive Polymers with Phase Transitions Caused by Cleavage
Abstract: Utilizing water-soluble anionic polymer conjugates derived from polyallylamine and phthalic acid with cleavage-induced phase transition property, a novel programmed upper critical solution temperature-type thermoresponsive polymer was developed. A side chain cleavage reaction in acidic aqueous media induces the intrinsic charge inversion of the polymer side chain from anion to cation. The polymer conjugates exhibit a thermoresponsive property as side chain cleavage proceeds under constant external conditions, and the phase boundary shifts as a result of the altered polymer composition. Phase transition takes place under fixed external conditions once the phase transition boundary eventually reaches the temperature under investigation. This study’s novel discovery introduces the idea of a time-programmed stimuli-responsive polymer with a cleavage-induced phase transition.
Keywords: thermoresponsive polymer; phase boundary; cleavage reaction
Paper Quality: SCOPUS / Web of Science Level Research Paper
Subject: Chemistry
Writer Experience: 20+ Years
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